The processor can access data words in memory in little-endian format or big-endian format. It always accesses code in little-endian format.
Little-endian is the default memory format for ARM processors.
The processor contains a configuration pin, BIGEND, that enables you to select either the little-endian or BE-8 big-endian format. This configuration pin is sampled on reset.
You cannot change endianness when out of reset.
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